IP Library Granted Patent US 12,191,139
Granted Patent B2
US 12,191,139 · App. 17/563,024 · Granted Jan 7, 2025

Selective molecular layer deposition of organic and hybrid organic-inorganic layers

Inventors: Tapash Chakraborty (Maharashtra, IN); Robert Jan Visser (Menlo Park, CA); Prerna Goradia (Mumbai, IN)
Assignee: Applied Materials, Inc.
H01L21/02118C23C16/45553H01L21/0228H01L21/02304H01L21/02312H01L21/3105B05D1/36B05D1/60
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Quick Facts
Patent No.
US 12,191,139
App. No.
17/563,024
Granted
Jan 7, 2025
Kind
B2
Abstract

Embodiments of the disclosure relate to methods of selectively depositing organic and hybrid organic/inorganic layers. More particularly, embodiments of the disclosure are directed to methods of modifying hydroxyl terminated surfaces for selective deposition of molecular layer organic and hybrid organic/inorganic films. Additional embodiments of the disclosure relate to cyclic compounds for use in molecular layer deposition processes.

Claims (12)

1. A method of depositing a film comprising:

providing a substrate comprising a first material having a hydrogen terminated surface and a second material having a hydroxyl terminated surface;

exposing the substrate to a modifying compound comprising a modifying species that reacts with the hydroxyl terminated surface of the second material to form a modified second surface on the second material; and

exposing the substrate to one or more deposition gases which react with the modified second surface of the second material to form a film on the second material,

wherein the modifying species has a general formula (RO) 3 Si-L-Si(OR) 3 where each R is independently selected from C1-C4 alkyl groups and L is an aromatic moiety or a carbon chain comprising 1 to 3 carbon atoms.

2. The method of claim 1 , wherein the first material comprises silicon and the second material comprises silicon oxide.

3. The method of claim 1 , wherein R consists essentially of methyl.

4. The method of claim 1 , wherein L is a phenyl group.

5. The method of claim 4 , wherein the phenyl group has the silicon atoms in a para position.

6. The method of claim 1 , wherein L is —(CH 2 ) 2 —.

7. The method of claim 1 , wherein L contains at least one double bond.

8. The method of claim 7 , wherein L is-CH═CH—.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 26, 2022
From: CHAKRABORTY, TAPASH; VISSER, ROBERT JAN; GORADIA, PRERNA SONTHALIA
To: APPLIED MATERIALS, INC.
Reel/Frame 058779/0461 →
Continuity (4)
Division 15986178 · May 22, 2018
Provisional Application 62547436 · Aug 18, 2017
Provisional Application 62512067 · May 28, 2017
Related Publication 20220130663A1 · Apr 28, 2022
References Cited (23)
US 20060183322A1 · Sandhu et al. · 2006 [cited by applicant]
US 20080199977A1 · Weigel · 2008 [cited by examiner]
US 20100123097A1 · Belfadhel et al. · 2010 [cited by applicant]
US 20120121932A1 · George et al. · 2012 [cited by applicant]
US 20130330482A1 · Leu et al. · 2013 [cited by applicant]
US 20140231968A1 · Gronheid · 2014 [cited by examiner]
US 20150021774A1 · Chiang et al. · 2015 [cited by applicant]
US 20160244581A1 · Brink et al. · 2016 [cited by applicant]
US 20160322213A1 · Thompson et al. · 2016 [cited by applicant]
EP 2818474A1 · 2014 [cited by applicant]
JP 2010012769A · 2010 [cited by applicant]
WO 2006097525A2 · 2006 [cited by applicant]
WO WO2010019125A1 · 2010 [cited by examiner]
Machine Translation of JP2010012769A, 15 pages. [cited by applicant]
PCT International Search Report and Written Opinion in PCT/US2018/033894 dated Sep. 21, 2018, 12 pages. [cited by applicant]
George, Steven M., et al., “Surface Chemistry for Molecular Layer Deposition of Organic and Hybrid Organic-Inorganic Polymers”, Accounts of Chemical Research, vol. 42, No. 4, Apr. 2009, pp. 498-508. [cited by applicant]
Haensch, Claudia , et al., “Chemical modification of self-assembled silane based monolayers by surface reactions”, Chem. Soc. Rev., 2010, 39, pp. 2323-2334. [cited by applicant]
Jiang, Ying-Bing , et al., “Sub-10 nm Thick Microporous Membranes Made by Plasma-Defined Atomic Layer Deposition of a Bridged Silsesquioxane Precursor”, J. Am. Chem. Soc. 2007, 129, 15446-15447. [cited by applicant]
Ju, Ling , et al., “Cyclic azasilanes as volatile and reactive precursors for atomic layer deposition of silicon dioxide”, J. Mater. Chem. C, 2016, 4, 4034-4039. [cited by applicant]
Ju, Ling , et al., “Molecular layer deposition using cyclic azasilanes, maleic anhydride, trimethylaluminum, and water”, J. Vac. Sci. Technol. A 35(1), Jan./Feb. 2017, 9 pages. [cited by applicant]
Maddox, Annalese F., et al., “Single Molecular Layer Adaption of Interfacial Surfaces by Cyclic Azasilane “Click-Chemistry””, Mater. Res. Soc. Symp. Proc. vol. 1793, 2015 Materials Research Society, 7 pages. [cited by applicant]
Sundberg, Pia , et al., “Organic and inorganic-organic thin film structures by molecular layer deposition: A review”, Beilstein J. Nanotechnol. 2014, 5, 1104-1136. [cited by applicant]
Van Bui, H. , et al., “Atomic and molecular layer deposition: off the beaten track”, Chem. Commun., 2017, 53, 45-71. [cited by applicant]