IP Library › Granted Patent US 12,671,082
Granted Patent B2
US 12,671,082 · App. 18/999,714 · Granted Jun 30, 2026

Electroactive materials for metal-ion batteries

Inventors: Charles A. Mason (Oxford, GB); Richard Gregory Taylor (Penarth, GB); James Farrell (Oxford, GB); William James Macklin (Wantage, GB)
Assignee: Nexeon Limited
H01M4/364H01M4/133H01M4/134H01M4/386H01M4/625H01M10/0525H01M2004/021H01M2004/027
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Quick Facts
Patent No.
US 12,671,082
App. No.
18/999,714
Filed
Dec 23, 2024
Granted
Jun 30, 2026
Kind
B2
Art Unit
1761
USPC
429/231.8
Abstract

This invention relates to particulate electroactive materials comprising a plurality of composite particles, wherein the composite particles comprise: (a) a porous carbon framework including micropores and/or mesopores having a total volume of at least 0.7 cm 3 /g, wherein at least half of the micropore/mesopore volume is in the form of pores having a diameter of no more than 5 nm; and (b) silicon located within the micropores and/or mesopores of the porous carbon framework in a defined amount relative to the volume of the micropores and/or mesopores.

Claims (46)

1 . A particulate material comprising a plurality of composite particles, wherein the composite particles comprise:

(a) a porous carbon framework comprising micropores and/or mesopores, wherein

the micropores and/or mesopores have a total pore volume as measured by gas adsorption of P 1 cm 3 /g, wherein P 1 has a value in the range from 0.7 to 1.4, and

the PD 50 pore diameter as measured by gas adsorption is no more than 4 nm;

the PD 90 pore diameter as measured by gas adsorption is no more than 15 nm; and

(b) a plurality of nanoscale silicon domains located within the micropores and/or mesopores of the porous carbon framework,

wherein

the weight ratio of silicon to the porous carbon framework in the composite particles is in the range from [0.5×P 1 to 1.3×P 1 ]:1;

the particulate material has a Z value of no more than 10% as determined by TGA analysis in air, in which Z=1.875×[(M f −M 800 )/M f ]×100%, in which M f is the mass of the TGA sample at completion of oxidation and M 800 is the mass of the TGA sample at 800° C.; and

the total oxygen content of the composite particles is less than 10 wt %.

2 . A particulate material according to claim 1 , wherein P 1 is in the range from 0.75 to 1.3.

3 . A particulate material according to claim 1 , wherein the PD 50 pore diameter of the porous carbon framework is no more than 3 nm.

4 . A particulate material according to claim 1 , wherein the PD 7 O pore diameter of the porous carbon framework is no more than 5 nm.

5 . A particulate material according to claim 1 , wherein the PD 95 pore diameter of the porous carbon framework is no more than 20 nm.

6 . A particulate material according to claim 1 , wherein the weight ratio of silicon to the porous carbon framework is in the range from [0.5×P 1 to 1.2×P 1 ]:1.

7 . A particulate material according to claim 1 , wherein at least a portion of the micropores and/or mesopores comprise void space that is fully enclosed by the silicon.

8 . A particulate material according to claim 1 , wherein at least 90 wt % of the silicon mass in the composite particles is located within the internal pore volume of the porous carbon framework.

9 . A particulate material according to claim 1 , wherein the porous carbon framework is obtained by the pyrolysis of plant biomass, lignocellulosic materials and fossil carbon sources.

10 . A particulate material according to claim 1 , wherein Z is no more than 5%.

11 . A particulate material according to claim 1 , wherein the composite particles have a D 50 particle diameter of no more than 20 μm.

12 . A particulate material according to claim 1 , wherein the composite particles have a D 10 particle diameter of at least 0.2 μm and a D 90 particle diameter of no more than 80 μm.

13 . A particulate material according to claim 1 , wherein the composite particles have a particle size distribution span of 5 or less.

14 . A particulate material according to claim 1 , wherein the composite particles have a BET surface area of no more than 150 m 2 /g.

15 . A particulate material according to claim 1 , having specific capacity on lithiation of 1200 to 2340 mAh/g.

16 . A composition comprising a particulate material according to claim 1 , and at least one other component selected from: (i) a binder; (ii) a conductive additive; and (iii) an additional particulate electroactive material.

17 . An electrode comprising a particulate material according to claim 1 , in electrical contact with a current collector.

18 . A rechargeable metal-ion battery comprising:

(i) an anode, wherein the anode comprises an electrode according to claim 17 ;

(ii) a cathode comprising a cathode active material capable of releasing and reabsorbing metal ions; and

(iii) an electrolyte between the anode and the cathode.

19 . A particulate material comprising a plurality of composite particles, wherein the composite particles comprise:

(a) a porous carbon framework comprising micropores and/or mesopores, wherein

the micropores and/or mesopores have a total pore volume as measured by gas adsorption of P 1 cm 3 /g, wherein P 1 has a value of no more than 1.4, and

the PD 7 O pore diameter as measured by gas adsorption is no more than 5 nm; and

(b) a plurality of nanoscale silicon domains located within the micropores and/or mesopores of the porous carbon framework,

wherein

the weight ratio of silicon to the porous carbon framework in the composite particles is in the range from [0.5×P 1 to 1.3×P 1 ]:1;

the particulate material has a Z value of no more than 10% as determined by TGA analysis in air, in which Z=1.875×[(M f −M 800 )/M f ]×100%, in which M f is the mass of the TGA sample at completion of oxidation and M 800 is the mass of the TGA sample at 800° C.; and

the composite particles have a particle size distribution span of 5 or less.

20 . A particulate material according to claim 19 , wherein the PD 7 O pore diameter as measured by gas adsorption is no more than 2 nm.

21 . A particulate material according to claim 19 , wherein the PD 50 pore diameter as measured by gas adsorption is no more than 2 nm, and Z is no more than 5%.

22 . A particulate material according to claim 19 , wherein:

the porous carbon framework comprises amorphous carbon;

the total volume of macropores in the porous carbon framework is P 2 cm 3 /g, wherein P 2 is no more than 0.1×P 1 ;

the silicon is amorphous silicon; and

the specific capacity of the particulate material on lithiation is 1200 to 2340 mAh/g.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 23, 2024
From: TAYLOR, RICHARD GREGORY
To: NEXEON LIMITED
Reel/Frame 069669/0209 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 23, 2024
From: MASON, CHARLES A.; FARRELL, JAMES; MACKLIN, WILLIAM JAMES
To: NEXEON LIMITED
Reel/Frame 069669/0289 →
Priority Claims (3)
GB 1818232 · Nov 8, 2018 · national
GB 1820736 · Dec 19, 2018 · national
GB 1912993 · Sep 9, 2019 · national
Continuity (3)
Continuation 17292241
Continuation In Part 16274182 · Feb 12, 2019
Related Publication 20250357467A1 · Nov 20, 2025
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